It is not the size of the aberrations alone that decides. Three things do: the aberration level, the purpose of the evaluation, and the computation conditions. In systems with large aberrations, where the rays land more or less decides the performance, so spot diagrams, ray aberration plots, geometric MTF and geometric encircled energy work well. As a system approaches the diffraction limit, ray spread no longer describes performance, and you move to diffraction-based metrics such as the point spread function and the Strehl ratio. Purpose matters too: whether you are asking about contrast, about the fraction of energy, or about how it actually looks changes the metric you choose. Computation conditions matter as well: depending on f-number, image plane tilt, exit pupil distortion and sampling density, the diffraction calculation itself may not hold.
There are several concrete guides on aberration level. On a spot diagram, if all the rays fall well inside the Airy disc, the system can be taken as diffraction limited. For diffraction-based MTF, switch to geometric MTF once the wavefront error exceeds about 10 waves. Image simulation switches automatically from a diffraction point spread to a geometric one at 20 times the diffraction limit. The Strehl ratio approximation from Zernike coefficients is only usable for monochromatic light and where the Strehl ratio is above about 0.10. These are guides: judge them together with the purpose of the evaluation and the computation conditions.